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Yes. Ravana used his sword against Jatayu. Ravana forcefully abducts Seetha in his air-chariot also known as Pushpaka Vimana. Finally, Seetha sees Jatayu, the eagle, and asks him to narrate her abduction to Rama. Jataayu confronts Ravana on hearing the wailing of Seetha. He boldly forestalls Ravana and his air-chariot in the sky itself, and as an elderly being he reviles Ravana from the viewpoint of righteousness befitting to kings, but of no avail.

That unexcelled bird of high refulgence then shattered Ravana's bow which is decorated with pearls and gemstones, and on which an arrow is admitted targeting the eagle, just by the pair of his bare feet.

When that demon of cruel actions has ruptured his wings that colossal eagle Jataayu immediately fell down to earth with a lessened life.

Yes. Ravana used his sword against Jatayu. Ravana forcefully abducts Seetha in his air-chariot also known as Pushpaka Vimana. Finally, Seetha sees Jatayu, the great vulture, and asks him to narrate her abduction to Rama. Jataayu confronts Ravana on hearing the wailing of Seetha. He boldly forestalls Ravana and his air-chariot in the sky itself, and as an elderly being he reviles Ravana from the viewpoint of righteousness befitting to kings, but of no avail.

That unexcelled bird of high refulgence then shattered Ravana's bow which is decorated with pearls and gemstones, and on which an arrow is admitted targeting the vulture, just by the pair of his bare feet.

When that demon of cruel actions has ruptured his wings that colossal vulture Jataayu immediately fell down to earth with a lessened life.

Ravana used the sword to kill/harm Jatayu who was forestalling him in the abduction of Seetha. This is clearly adharma. Moreover there is no mention of using a sword by Ravana other than this incident. So this sword should be the sword Chandrahasa. So the sword should have returned to Lord Shiva.

Conclusion:

The sword used against Jatayu is none other than Chandrahasa. As the sword has returned to Lord Shiva after this incident, there is no mention of him using a sword against Rama in the final battle.

Ravana used the sword to kill/harm Jatayu who was forestalling him in the abduction of Seetha. This is clearly adharma.

After this incident, there is only one incident where Ravana uses a sword but neither the name is mentioned nor the origin of it.

उत्प्लुत्य गुणसम्पन्नं विमलाम्बरवर्चसं |
निष्पपात स वेगेन सभायाः सचिवैर्वृतः || 6-92-39

रावणः पुत्रशोकेन भृशमाकुलचेतनः |
संक्रुद्धः खड्गमादाय सहसा यत्र मैथिली || 6-92-40

The enraged Ravana, who was very much agitated in mind because of the grief for his son's death, springing up suddenly and taking his excellent sword, having the dazzle of a clear sky, sallied forth from the assembly hall along with his ministers swiftly and quickly to the place where Seetha was.

He thought of killing Seetha using his sword but got pacified later.

It was not explicitly mentioned that this sword is Chandrahasa.

Conclusion: The sword used against Jatayu should possibly be Chandrahasa. The sword would have returned to Lord Shiva after this Jatayu incident. As the sword has returned, there is no mention of him using a sword against Rama in the final battle. We cannot dismiss claim of using a sword in the battle saying it is a distance battle. Sword was used against Sugriva by the demon Virupaksha.

Ravana used the sword to kill/harm Jatayu who was forestalling him in the abduction of Seetha. This is clearly adharma. So the sword might have returned to Lord Shiva.

Ravana used the sword to kill/harm Jatayu who was forestalling him in the abduction of Seetha. This is clearly adharma. Moreover there is no mention of using a sword by Ravana other than this incident. So this sword should be the sword Chandrahasa. So the sword should have returned to Lord Shiva.